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  • Syntheses, structures, and (1)H, (13)C{(1)H} and (119)Sn{(1)H} NMR chemical shifts of a family of trimethyltin alkoxide, amide, halide and cyclopentadienyl compounds.

Syntheses, structures, and (1)H, (13)C{(1)H} and (119)Sn{(1)H} NMR chemical shifts of a family of trimethyltin alkoxide, amide, halide and cyclopentadienyl compounds.

Dalton transactions (Cambridge, England : 2003) (2015-08-22)
Alejandro G Lichtscheidl, Michael T Janicke, Brian L Scott, Andrew T Nelson, Jaqueline L Kiplinger
ABSTRACT

The synthesis and full characterization, including Nuclear Magnetic Resonance (NMR) data ((1)H, (13)C{(1)H} and (119)Sn{(1)H}), for a series of Me3SnX (X = O-2,6-(t)Bu2C6H3 (), (Me3Sn)N(2,6-(i)Pr2C6H3) (), NH-2,4,6-(t)Bu3C6H2 (), N(SiMe3)2 (), NEt2, C5Me5 (), Cl, Br, I, and SnMe3) compounds in benzene-d6, toluene-d8, dichloromethane-d2, chloroform-d1, acetonitrile-d3, and tetrahydrofuran-d8 are reported. The X-ray crystal structures of Me3Sn(O-2,6-(t)Bu2C6H3) (), Me3Sn(O-2,6-(i)Pr2C6H3) (), and (Me3Sn)(NH-2,4,6-(t)Bu3C6H2) () are also presented. These compiled data complement existing literature data and ease the characterization of these compounds by routine NMR experiments.

MATERIALS
Product Number
Brand
Product Description

Sigma-Aldrich
Aluminum oxide, mesoporous, MSU-X (wormhole), average pore size 3.8 nm
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Tetrahydrofuran-d8, ≥99.5 atom % D, contains 0.03 % (v/v) TMS
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Tetrahydrofuran-d8, ≥99.5 atom % D, contains 1 % (v/v) TMS
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Acetonitrile-d3, 96-97 atom % D, D2O 15-20 %
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Acetonitrile-d3, ≥99.8 atom % D
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Tetrahydrofuran-d8, ≥99.5 atom % D
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Tetrahydrofuran-d8, ≥99.5 atom % D
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Acetonitrile-d3, "100%", 99.96 atom % D
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Acetonitrile-d3, 99.8 atom % D, contains 1 % (v/v) TMS
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Acetonitrile-d3, 99.8 atom % D, contains 0.03 % (v/v) TMS
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Acetonitrile-d3, ≥99.8 atom % D, anhydrous
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Dichloromethane-d2, 99.9 atom % D, contains 0.1 % (v/v) TMS
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Sigma-Aldrich
Benzene-D6, anhydrous, ≥99.6 atom % D
Sigma-Aldrich
Dichloromethane-d2, "100%", 99.96 atom % D
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Benzene-D6, 99.6 atom % D
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Sigma-Aldrich
Toluene-d8, 99 atom % D, contains 0.03 % (v/v) TMS
Sigma-Aldrich
Dichloromethane-d2, ≥99.5 atom % D, contains 0.03 % (v/v) TMS
Sigma-Aldrich
Dichloromethane-d2, 99.5 atom % D